This dataset presents modelled estimates of soil nitrogen concentration (% dry weight soil) at 1km2 resolution across Great Britain. A Generalized Additive Model approach was used with Countryside Survey soil nitrogen data from 2007 and including climate, atmospheric deposition, habitat, soil and spatial predictors. The model is based on soil nitrogen data from 913 locations across Great Britain and is representative of 0-15 cm soil depth. Soil N concentration was determined using a total elemental analyser. The Countryside Survey looks at a range of physical, chemical and biological properties of the topsoil from a representative sample of habitats across the UK. This work was supported by the Natural Environment Research Council award number NE/R016429/1 as part of the UK-SCAPE programme delivering National Capability.